Articles | Volume 17, issue 5
https://doi.org/10.5194/cp-17-2119-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/cp-17-2119-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
New insights into the ∼ 74 ka Toba eruption from sulfur isotopes of polar ice cores
School Of Earth And Environmental Sciences, University Of St Andrews, St Andrews, United Kingdom
Andrea Burke
School Of Earth And Environmental Sciences, University Of St Andrews, St Andrews, United Kingdom
William Hutchison
School Of Earth And Environmental Sciences, University Of St Andrews, St Andrews, United Kingdom
Mika Kohno
Geoscience Center (GZG), Department of Geochemistry, Georg August Universität Göttingen, Göttingen, Germany
Kathryn A. Moore
Department Of Atmospheric Science, Colorado State University, Fort Collins, Colorado, USA
Joel Savarino
Institut Des Géosciences De L'environnement, Grenoble, France
Emily A. Doyle
Department Of Earth Sciences, University Of Cambridge, Cambridge, United Kingdom
Sue Mahony
School Of Earth Sciences, University Of Bristol, Bristol, United Kingdom
Sepp Kipfstuhl
Alfred Wegener Institute, Bremerhaven, Germany
James W. B. Rae
School Of Earth And Environmental Sciences, University Of St Andrews, St Andrews, United Kingdom
Robert C. J. Steele
School Of Earth And Environmental Sciences, University Of St Andrews, St Andrews, United Kingdom
R. Stephen J. Sparks
School Of Earth Sciences, University Of Bristol, Bristol, United Kingdom
Eric W. Wolff
Department Of Earth Sciences, University Of Cambridge, Cambridge, United Kingdom
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Eric W. Wolff, Andrea Burke, Laura Crick, Emily A. Doyle, Helen M. Innes, Sue H. Mahony, James W. B. Rae, Mirko Severi, and R. Stephen J. Sparks
Clim. Past, 19, 23–33, https://doi.org/10.5194/cp-19-23-2023, https://doi.org/10.5194/cp-19-23-2023, 2023
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Large volcanic eruptions leave an imprint of a spike of sulfate deposition that can be measured in ice cores. Here we use a method that logs the number and size of large eruptions recorded in an Antarctic core in a consistent way through the last 200 000 years. The rate of recorded eruptions is variable but shows no trends. In particular, there is no increase in recorded eruptions during deglaciation periods. This is consistent with most recorded eruptions being from lower latitudes.
Agnese Petteni, Mathieu Casado, Christophe Leroy-Dos Santos, Amaelle Landais, Niels Dutrievoz, Cécile Agosta, Pete D. Akers, Joel Savarino, Andrea Spolaor, Massimo Frezzotti, and Barbara Stenni
EGUsphere, https://doi.org/10.5194/egusphere-2025-3188, https://doi.org/10.5194/egusphere-2025-3188, 2025
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We investigated the isotopic composition of surface snow in a previously unexplored region of East Antarctica to understand how differences in air mass origin influence its variability. By comparing observations with model data, we validated the model and quantified the impact of post-depositional processes at the snow–atmosphere interface. Our results offer valuable insights for reconstructing past temperatures from ice cores.
Adrien Ooms, Mathieu Casado, Ghislain Picard, Laurent Arnaud, Maria Hörhold, Andrea Spolaor, Rita Traversi, Joel Savarino, Patrick Ginot, Pete Akers, Birthe Twarloh, and Valérie Masson-Delmotte
EGUsphere, https://doi.org/10.5194/egusphere-2025-3259, https://doi.org/10.5194/egusphere-2025-3259, 2025
This preprint is open for discussion and under review for The Cryosphere (TC).
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This work presents a new approach to the estimation of accumulation rates at Concordia Station, East-Antarctica, for the last 20 years, from a new data set of chemical tracers and snow micro-scale properties measured in a snow trench. Multi-annual and meter to decameter scale variability of accumulation rates are compared again in-situ measurements of surface laser scanner and stake farm, with very good agreement. This further constrains SMB estimation for Antarctica at high temporal resolution.
Amy Constance Faith King, Thomas Keith Bauska, Amaelle Landais, Carlos Martin, and Eric William Wolff
EGUsphere, https://doi.org/10.5194/egusphere-2025-3305, https://doi.org/10.5194/egusphere-2025-3305, 2025
This preprint is open for discussion and under review for Climate of the Past (CP).
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We show how measurements of nitrogen isotopes in Antarctic ice core records can be used to show dramatic thinning of an ice sheet during ice mass changes in the Holocene. Combining such measurements with proxies for ice sheet elevation could be a powerful tool for constraining the history of ice dynamics at sites which are sensitive to rapid changes, and could contribute to constraining ice sheet models.
Lison Soussaintjean, Jochen Schmitt, Joël Savarino, J. Andy Menking, Edward J. Brook, Barbara Seth, Vladimir Lipenkov, Thomas Röckmann, and Hubertus Fischer
EGUsphere, https://doi.org/10.5194/egusphere-2025-3108, https://doi.org/10.5194/egusphere-2025-3108, 2025
This preprint is open for discussion and under review for Biogeosciences (BG).
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Nitrous oxide (N2O) produced in dust-rich Antarctic ice complicates the reconstruction of past atmospheric levels from ice core records. Using isotope analysis, we show that N2O forms from two nitrogen precursors, one being nitrate. For the first time, we demonstrate that the site preference (SP) of N2O reflects the isotopic difference between these precursors, not the production pathway, which challenges the common interpretation of SP.
Filip Pastierovic, Roberto Grilli, Nicolas Caillon, and Joel Savarino
EGUsphere, https://doi.org/10.5194/egusphere-2025-3115, https://doi.org/10.5194/egusphere-2025-3115, 2025
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The development of an open detector based on absorption spectroscopy, enhanced by high-reflectivity mirrors, for the simultaneous measurement of NO2, IO, and CHOCHO is reported. The instrument shows good correlation with a closed system during both indoor and outdoor measurements. An open system is able to measure NO2, IO, and CHOCHO with high precision.
Zhao Wei, Shohei Hattori, Asuka Tsuruta, Zhuang Jiang, Sakiko Ishino, Koji Fujita, Sumito Matoba, Lei Geng, Alexis Lamothe, Ryu Uemura, Naohiro Yoshida, Joel Savarino, and Yoshinori Iizuka
Atmos. Chem. Phys., 25, 5727–5742, https://doi.org/10.5194/acp-25-5727-2025, https://doi.org/10.5194/acp-25-5727-2025, 2025
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Nitrate isotope records in ice cores reveal changes in NOₓ emissions and atmospheric oxidation chemistry driven by human activity. However, UV-driven postdepositional processes can alter nitrate in snow, making snow accumulation rates critical for preserving these records. This study examines nitrate isotopes in a southeastern Greenland ice core, where high snow accumulation minimizes these effects, providing a reliable archive of atmospheric nitrogen cycling.
Felix S. L. Ng, Rachael H. Rhodes, Tyler J. Fudge, and Eric W. Wolff
EGUsphere, https://doi.org/10.5194/egusphere-2025-1566, https://doi.org/10.5194/egusphere-2025-1566, 2025
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Impurity diffusion in ice causes loss of climate history. We give a new method of finding the diffusion rate from ice-core records. Its use on sulphate data from the EPICA Dome C core reveals rapid diffusion in snow that suggests H2SO4 vapour diffusion in air pores, and much slower diffusion in the ice below that indicates signal relocation between crystal interfaces. We estimate a maximum sulphate diffusion length of 2 cm for ice 1–2 Myr old sought by the ice-coring projects on Little Dome C.
Niklas Kappelt, Eric Wolff, Marcus Christl, Christof Vockenhuber, Philip Gautschi, and Raimund Muscheler
EGUsphere, https://doi.org/10.5194/egusphere-2025-1780, https://doi.org/10.5194/egusphere-2025-1780, 2025
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By measuring the radioactive decay of atmospherically produced 36Cl and 10Be in an ice core drilled in West Antarctica, we were able to determine the age of the deepest sample close to bedrock to be about 550 thousand years old. This means that the ice in this location, known as Skytrain Ice Rise, has survived several warm periods in the past, which occur about every 100 thousand years.
Kathryn A. Moore, Thomas C. J. Hill, Chamika K. Madawala, Raymond J. Leibensperger III, Samantha Greeney, Christopher D. Cappa, M. Dale Stokes, Grant B. Deane, Christopher Lee, Alexei V. Tivanski, Kimberly A. Prather, and Paul J. DeMott
Atmos. Chem. Phys., 25, 3131–3159, https://doi.org/10.5194/acp-25-3131-2025, https://doi.org/10.5194/acp-25-3131-2025, 2025
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This article presents results from the first study in a new wind–wave channel at the Scripps Institution of Oceanography. The experiment tested how wind over the ocean surface influences production of sea spray particles, which are important for radiative forcing and cloud formation in the atmosphere. We found that particle concentration and chemical composition varied with wind speed and that variations were driven by changes in wind and wave breaking rather than seawater biology or chemistry.
Florian Painer, Sepp Kipfstuhl, Martyn Drury, Tsutomu Uchida, Johannes Freitag, and Ilka Weikusat
EGUsphere, https://doi.org/10.5194/egusphere-2025-633, https://doi.org/10.5194/egusphere-2025-633, 2025
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Air clathrate hydrates trap ancient air in the deeper part of ice sheets. We use digital microscopy and automated image analysis to investigate the evolution of number, size and shape of air clathrate hydrates from 1250 m depth to the bottom of the ice sheet. We confirm the previously found relation of changes in number and size with past climate and find a connection of their shape to changes in ice deformation. The results will help to better understand air clathrate hydrates in deep ice.
Brice Barret, Patrice Medina, Natalie Brett, Roman Pohorsky, Kathy S. Law, Slimane Bekki, Gilberto J. Fochesatto, Julia Schmale, Steve R. Arnold, Andrea Baccarini, Maurizio Busetto, Meeta Cesler-Maloney, Barbara D'Anna, Stefano Decesari, Jingqiu Mao, Gianluca Pappaccogli, Joel Savarino, Federico Scoto, and William R. Simpson
Atmos. Meas. Tech., 18, 1163–1184, https://doi.org/10.5194/amt-18-1163-2025, https://doi.org/10.5194/amt-18-1163-2025, 2025
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The Fairbanks area experiences severe pollution episodes in winter because of enhanced emissions of pollutants trapped near the surface by strong temperature inversions. Low-cost sensors were deployed on board a car and a tethered balloon to measure the concentrations of gaseous pollutants (CO, O3, and NOx) in Fairbanks during winter 2022. Data calibration with reference measurements and machine learning methods enabled us to document pollution at the surface and power plant plumes aloft.
Natalie Brett, Kathy S. Law, Steve R. Arnold, Javier G. Fochesatto, Jean-Christophe Raut, Tatsuo Onishi, Robert Gilliam, Kathleen Fahey, Deanna Huff, George Pouliot, Brice Barret, Elsa Dieudonné, Roman Pohorsky, Julia Schmale, Andrea Baccarini, Slimane Bekki, Gianluca Pappaccogli, Federico Scoto, Stefano Decesari, Antonio Donateo, Meeta Cesler-Maloney, William Simpson, Patrice Medina, Barbara D'Anna, Brice Temime-Roussel, Joel Savarino, Sarah Albertin, Jingqiu Mao, Becky Alexander, Allison Moon, Peter F. DeCarlo, Vanessa Selimovic, Robert Yokelson, and Ellis S. Robinson
Atmos. Chem. Phys., 25, 1063–1104, https://doi.org/10.5194/acp-25-1063-2025, https://doi.org/10.5194/acp-25-1063-2025, 2025
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Processes influencing dispersion of local anthropogenic pollution in Arctic wintertime are investigated with Lagrangian dispersion modelling. Simulated power plant plume rise that considers temperature inversion layers improves results compared to observations (interior Alaska). Modelled surface concentrations are improved by representation of vertical mixing and emission estimates. Large increases in diesel vehicle emissions at temperatures reaching −35°C are required to reproduce observed NOx.
Agnese Petteni, Elise Fourré, Elsa Gautier, Azzurra Spagnesi, Roxanne Jacob, Pete D. Akers, Daniele Zannoni, Jacopo Gabrieli, Olivier Jossoud, Frédéric Prié, Amaëlle Landais, Titouan Tcheng, Barbara Stenni, Joel Savarino, Patrick Ginot, and Mathieu Casado
EGUsphere, https://doi.org/10.5194/egusphere-2024-3335, https://doi.org/10.5194/egusphere-2024-3335, 2025
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Our research compares three CFA-CRDS systems from Venice, Paris, and Grenoble for measuring water isotopes in ice cores, crucial for reconstructing past climate. We quantify each system’s mixing and measurement noise effects, which impact the achievable resolution of isotope continuous records. Our findings reveal specific configurations and procedures to enhance measurement accuracy, providing a framework to optimise water isotope analysis.
Amna Ijaz, Brice Temime-Roussel, Benjamin Chazeau, Sarah Albertin, Stephen R. Arnold, Brice Barrett, Slimane Bekki, Natalie Brett, Meeta Cesler-Maloney, Elsa Dieudonne, Kayane K. Dingilian, Javier G. Fochesatto, Jingqiu Mao, Allison Moon, Joel Savarino, William Simpson, Rodney J. Weber, Kathy S. Law, and Barbara D'Anna
EGUsphere, https://doi.org/10.5194/egusphere-2024-3789, https://doi.org/10.5194/egusphere-2024-3789, 2024
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Fairbanks is among the most polluted cities with the highest particulate matter (PM) levels in the US during winters. Highly time-resolved measurements of the sub-micron PM elucidated residential heating with wood and oil and hydrocarbon-like organics from traffic, as well as sulphur-containing organic aerosol, to be the key pollution sources. Remarkable differences existed between complementary instruments, warranting the deployment of multiple tools at sites with wide-ranging influences.
Helene Hoffmann, Jason Day, Rachael H. Rhodes, Mackenzie Grieman, Jack Humby, Isobel Rowell, Christoph Nehrbass-Ahles, Robert Mulvaney, Sally Gibson, and Eric Wolff
The Cryosphere, 18, 4993–5013, https://doi.org/10.5194/tc-18-4993-2024, https://doi.org/10.5194/tc-18-4993-2024, 2024
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Ice cores are archives of past atmospheric conditions. In deep and old ice, the layers containing this information get thinned to the millimetre scale or below. We installed a setup for high-resolution (182 μm) chemical impurity measurements in ice cores using the laser ablation technique at the University of Cambridge. In a first application to the Skytrain ice core from Antarctica, we discuss the potential to detect fine-layered structures in ice up to an age of 26 000 years.
Nicolas Stoll, Ilka Weikusat, Daniela Jansen, Paul Bons, Kyra Darányi, Julien Westhoff, Mária-Gema Llorens, David Wallis, Jan Eichler, Tomotaka Saruya, Tomoyuki Homma, Martyn Drury, Frank Wilhelms, Sepp Kipfstuhl, Dorthe Dahl-Jensen, and Johanna Kerch
EGUsphere, https://doi.org/10.5194/egusphere-2024-2653, https://doi.org/10.5194/egusphere-2024-2653, 2024
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A better understanding of ice flow requires more observational data. The EastGRIP core is the first ice core through an active ice stream. We discuss crystal orientation data to determine the present deformation regimes. A comparison with other deep ice cores shows the unique properties of EastGRIP and that deep ice originates from the Eemian. We further show that the overall plug flow of NEGIS is characterised by many small-scale variations, which remain to be considered in ice-flow models.
Rachael H. Rhodes, Yvan Bollet-Quivogne, Piers Barnes, Mirko Severi, and Eric W. Wolff
Clim. Past, 20, 2031–2043, https://doi.org/10.5194/cp-20-2031-2024, https://doi.org/10.5194/cp-20-2031-2024, 2024
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Some ionic components slowly move through glacier ice by diffusion, but the rate of this diffusion, its exact mechanism(s), and the factors that might influence it are poorly understood. In this study, we model how peaks in sulfate, deposited at Dome C on the Antarctic ice sheet after volcanic eruptions, change with depth and time. We find that the sulfate diffusion rate in ice is relatively fast in young ice near the surface, but the rate is markedly reduced over time.
Dorothea Elisabeth Moser, Elizabeth R. Thomas, Christoph Nehrbass-Ahles, Anja Eichler, and Eric Wolff
The Cryosphere, 18, 2691–2718, https://doi.org/10.5194/tc-18-2691-2024, https://doi.org/10.5194/tc-18-2691-2024, 2024
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Increasing temperatures worldwide lead to more melting of glaciers and ice caps, even in the polar regions. This is why ice-core scientists need to prepare to analyse records affected by melting and refreezing. In this paper, we present a summary of how near-surface melt forms, what structural imprints it leaves in snow, how various signatures used for ice-core climate reconstruction are altered, and how we can still extract valuable insights from melt-affected ice cores.
V. Holly L. Winton, Robert Mulvaney, Joel Savarino, Kyle R. Clem, and Markus M. Frey
Clim. Past, 20, 1213–1232, https://doi.org/10.5194/cp-20-1213-2024, https://doi.org/10.5194/cp-20-1213-2024, 2024
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In 2018, a new 120 m ice core was drilled in a region located under the Antarctic ozone hole. We present the first results including a 1300-year record of snow accumulation and aerosol chemistry. We investigate the aerosol and moisture source regions and atmospheric processes related to the ice core record and discuss what this means for developing a record of past ultraviolet radiation and ozone depletion using the stable isotopic composition of nitrate measured in the same ice core.
Zhuang Jiang, Becky Alexander, Joel Savarino, and Lei Geng
Atmos. Chem. Phys., 24, 4895–4914, https://doi.org/10.5194/acp-24-4895-2024, https://doi.org/10.5194/acp-24-4895-2024, 2024
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Ice-core nitrate could track the past atmospheric NOx and oxidant level, but its interpretation is hampered by the post-depositional processing. In this work, an inverse model was developed and tested against two polar sites and was shown to well reproduce the observed nitrate signals in snow and atmosphere, suggesting that the model can properly correct for the effect of post-depositional processing. This model offers a very useful tool for future studies on ice-core nitrate records.
Larissa Lacher, Michael P. Adams, Kevin Barry, Barbara Bertozzi, Heinz Bingemer, Cristian Boffo, Yannick Bras, Nicole Büttner, Dimitri Castarede, Daniel J. Cziczo, Paul J. DeMott, Romy Fösig, Megan Goodell, Kristina Höhler, Thomas C. J. Hill, Conrad Jentzsch, Luis A. Ladino, Ezra J. T. Levin, Stephan Mertes, Ottmar Möhler, Kathryn A. Moore, Benjamin J. Murray, Jens Nadolny, Tatjana Pfeuffer, David Picard, Carolina Ramírez-Romero, Mickael Ribeiro, Sarah Richter, Jann Schrod, Karine Sellegri, Frank Stratmann, Benjamin E. Swanson, Erik S. Thomson, Heike Wex, Martin J. Wolf, and Evelyn Freney
Atmos. Chem. Phys., 24, 2651–2678, https://doi.org/10.5194/acp-24-2651-2024, https://doi.org/10.5194/acp-24-2651-2024, 2024
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Aerosol particles that trigger ice formation in clouds are important for the climate system but are very rare in the atmosphere, challenging measurement techniques. Here we compare three cloud chambers and seven methods for collecting aerosol particles on filters for offline analysis at a mountaintop station. A general good agreement of the methods was found when sampling aerosol particles behind a whole air inlet, supporting their use for obtaining data that can be implemented in models.
Sarah Albertin, Joël Savarino, Slimane Bekki, Albane Barbero, Roberto Grilli, Quentin Fournier, Irène Ventrillard, Nicolas Caillon, and Kathy Law
Atmos. Chem. Phys., 24, 1361–1388, https://doi.org/10.5194/acp-24-1361-2024, https://doi.org/10.5194/acp-24-1361-2024, 2024
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This study reports the first simultaneous records of oxygen (Δ17O) and nitrogen (δ15N) isotopes in nitrogen dioxide (NO2) and nitrate (NO3−). These data are combined with atmospheric observations to explore sub-daily N reactive chemistry and quantify N fractionation effects in an Alpine winter city. The results highlight the necessity of using Δ17O and δ15N in both NO2 and NO3− to avoid biased estimations of NOx sources and fates from NO3− isotopic records in urban winter environments.
Ryan J. Patnaude, Kathryn A. Moore, Russell J. Perkins, Thomas C. J. Hill, Paul J. DeMott, and Sonia M. Kreidenweis
Atmos. Chem. Phys., 24, 911–928, https://doi.org/10.5194/acp-24-911-2024, https://doi.org/10.5194/acp-24-911-2024, 2024
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In this study we examined the effect of atmospheric aging on sea spray aerosols (SSAs) to form ice and how newly formed secondary marine aerosols (SMAs) may freeze at cirrus temperatures (< −38 °C). Results show that SSAs freeze at different relative humidities (RHs) depending on the temperature and that the ice-nucleating ability of SSA was not hindered by atmospheric aging. SMAs are shown to freeze at high RHs and are likely inefficient at forming ice at cirrus temperatures.
Alexis Lamothe, Joel Savarino, Patrick Ginot, Lison Soussaintjean, Elsa Gautier, Pete D. Akers, Nicolas Caillon, and Joseph Erbland
Atmos. Meas. Tech., 16, 4015–4030, https://doi.org/10.5194/amt-16-4015-2023, https://doi.org/10.5194/amt-16-4015-2023, 2023
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Ammonia is a reactive gas in our atmosphere that is key in air quality issues. Assessing its emissions and how it reacts is a hot topic that can be addressed from the past. Stable isotopes (the mass of the molecule) measured in ice cores (glacial archives) can teach us a lot. However, the concentrations in ice cores are very small. We propose a protocol to limit the contamination and apply it to one ice core drilled in Mont Blanc, describing the opportunities our method brings.
Isobel Rowell, Carlos Martin, Robert Mulvaney, Helena Pryer, Dieter Tetzner, Emily Doyle, Hara Madhav Talasila, Jilu Li, and Eric Wolff
Clim. Past, 19, 1699–1714, https://doi.org/10.5194/cp-19-1699-2023, https://doi.org/10.5194/cp-19-1699-2023, 2023
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We present an age scale for a new type of ice core from a vulnerable region in West Antarctic, which is lacking in longer-term (greater than a few centuries) ice core records. The Sherman Island core extends to greater than 1 kyr. We provide modelling evidence for the potential of a 10 kyr long core. We show that this new type of ice core can be robustly dated and that climate records from this core will be a significant addition to existing regional climate records.
Sune Olander Rasmussen, Dorthe Dahl-Jensen, Hubertus Fischer, Katrin Fuhrer, Steffen Bo Hansen, Margareta Hansson, Christine S. Hvidberg, Ulf Jonsell, Sepp Kipfstuhl, Urs Ruth, Jakob Schwander, Marie-Louise Siggaard-Andersen, Giulia Sinnl, Jørgen Peder Steffensen, Anders M. Svensson, and Bo M. Vinther
Earth Syst. Sci. Data, 15, 3351–3364, https://doi.org/10.5194/essd-15-3351-2023, https://doi.org/10.5194/essd-15-3351-2023, 2023
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Timescales are essential for interpreting palaeoclimate data. The data series presented here were used for annual-layer identification when constructing the timescales named the Greenland Ice-Core Chronology 2005 (GICC05) and the revised version GICC21. Hopefully, these high-resolution data sets will be useful also for other purposes.
Robert Mulvaney, Eric W. Wolff, Mackenzie M. Grieman, Helene H. Hoffmann, Jack D. Humby, Christoph Nehrbass-Ahles, Rachael H. Rhodes, Isobel F. Rowell, Frédéric Parrenin, Loïc Schmidely, Hubertus Fischer, Thomas F. Stocker, Marcus Christl, Raimund Muscheler, Amaelle Landais, and Frédéric Prié
Clim. Past, 19, 851–864, https://doi.org/10.5194/cp-19-851-2023, https://doi.org/10.5194/cp-19-851-2023, 2023
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We present an age scale for a new ice core drilled at Skytrain Ice Rise, an ice rise facing the Ronne Ice Shelf in Antarctica. Various measurements in the ice and air phases are used to match the ice core to other Antarctic cores that have already been dated, and a new age scale is constructed. The 651 m ice core includes ice that is confidently dated to 117 000–126 000 years ago, in the last interglacial. Older ice is found deeper down, but there are flow disturbances in the deeper ice.
Simone Ventisette, Samuele Baldini, Claudio Artoni, Silvia Becagli, Laura Caiazzo, Barbara Delmonte, Massimo Frezzotti, Raffaello Nardin, Joel Savarino, Mirko Severi, Andrea Spolaor, Barbara Stenni, and Rita Traversi
EGUsphere, https://doi.org/10.5194/egusphere-2023-393, https://doi.org/10.5194/egusphere-2023-393, 2023
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The paper reports the spatial variability of concentration and fluxes of chemical impurities in superficial snow over unexplored area of the East Antarctic ice sheet. Pinatubo and Puyehue-Cordón Caulle volcanic eruptions in non-sea salt sulfate and dust snow pits record were used to achieve the accumulation rates. Deposition (wet, dry and uptake from snow surface) and post deposition processes are constrained. These knowledges are fundamental in Antarctic ice cores stratigraphies interpretation.
David A. Hodell, Simon J. Crowhurst, Lucas Lourens, Vasiliki Margari, John Nicolson, James E. Rolfe, Luke C. Skinner, Nicola C. Thomas, Polychronis C. Tzedakis, Maryline J. Mleneck-Vautravers, and Eric W. Wolff
Clim. Past, 19, 607–636, https://doi.org/10.5194/cp-19-607-2023, https://doi.org/10.5194/cp-19-607-2023, 2023
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We produced a 1.5-million-year-long history of climate change at International Ocean Discovery Program Site U1385 of the Iberian margin, a well-known location for rapidly accumulating sediments on the seafloor. Our record demonstrates that longer-term orbital changes in Earth's climate were persistently overprinted by abrupt millennial-to-centennial climate variability. The occurrence of abrupt climate change is modulated by the slower variations in Earth's orbit and climate background state.
Romilly Harris Stuart, Anne-Katrine Faber, Sonja Wahl, Maria Hörhold, Sepp Kipfstuhl, Kristian Vasskog, Melanie Behrens, Alexandra M. Zuhr, and Hans Christian Steen-Larsen
The Cryosphere, 17, 1185–1204, https://doi.org/10.5194/tc-17-1185-2023, https://doi.org/10.5194/tc-17-1185-2023, 2023
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This empirical study uses continuous daily measurements from the Greenland Ice Sheet to document changes in surface snow properties. Consistent changes in snow isotopic composition are observed in the absence of deposition due to surface processes, indicating the isotopic signal of deposited precipitation is not always preserved. Our observations have potential implications for the interpretation of water isotopes in ice cores – historically assumed to reflect isotopic composition at deposition.
Eric W. Wolff, Andrea Burke, Laura Crick, Emily A. Doyle, Helen M. Innes, Sue H. Mahony, James W. B. Rae, Mirko Severi, and R. Stephen J. Sparks
Clim. Past, 19, 23–33, https://doi.org/10.5194/cp-19-23-2023, https://doi.org/10.5194/cp-19-23-2023, 2023
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Large volcanic eruptions leave an imprint of a spike of sulfate deposition that can be measured in ice cores. Here we use a method that logs the number and size of large eruptions recorded in an Antarctic core in a consistent way through the last 200 000 years. The rate of recorded eruptions is variable but shows no trends. In particular, there is no increase in recorded eruptions during deglaciation periods. This is consistent with most recorded eruptions being from lower latitudes.
Pete D. Akers, Joël Savarino, Nicolas Caillon, Olivier Magand, and Emmanuel Le Meur
Atmos. Chem. Phys., 22, 15637–15657, https://doi.org/10.5194/acp-22-15637-2022, https://doi.org/10.5194/acp-22-15637-2022, 2022
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Nitrate isotopes in Antarctic ice do not preserve the seasonal isotopic cycles of the atmosphere, which limits their use to study the past. We studied nitrate along an 850 km Antarctic transect to learn how these cycles are changed by sunlight-driven chemistry in the snow. Our findings suggest that the snow accumulation rate and other environmental signals can be extracted from nitrate with the right sampling and analytical approaches.
Jessica G. M. Crumpton-Banks, Thomas Tanner, Ivan Hernández Almeida, James W. B. Rae, and Heather Stoll
Biogeosciences, 19, 5633–5644, https://doi.org/10.5194/bg-19-5633-2022, https://doi.org/10.5194/bg-19-5633-2022, 2022
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Past ocean carbon is reconstructed using proxies, but it is unknown whether preparing ocean sediment for one proxy might damage the data given by another. We have tested whether the extraction of an organic proxy archive from sediment samples impacts the geochemistry of tiny shells also within the sediment. We find no difference in shell geochemistry between samples which come from treated and untreated sediment. This will help us to maximize scientific return from valuable sediment samples.
Yanzhi Cao, Zhuang Jiang, Becky Alexander, Jihong Cole-Dai, Joel Savarino, Joseph Erbland, and Lei Geng
Atmos. Chem. Phys., 22, 13407–13422, https://doi.org/10.5194/acp-22-13407-2022, https://doi.org/10.5194/acp-22-13407-2022, 2022
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We investigate the potential of ice-core preserved nitrate isotopes as proxies of stratospheric ozone variability by measuring nitrate isotopes in a shallow ice core from the South Pole. The large variability in the snow accumulation rate and its slight increase after the 1970s masked any signals caused by the ozone hole. Moreover, the nitrate oxygen isotope decrease may reflect changes in the atmospheric oxidation environment in the Southern Ocean.
Andrea Bevilacqua, Alvaro Aravena, Willy Aspinall, Antonio Costa, Sue Mahony, Augusto Neri, Stephen Sparks, and Brittain Hill
Nat. Hazards Earth Syst. Sci., 22, 3329–3348, https://doi.org/10.5194/nhess-22-3329-2022, https://doi.org/10.5194/nhess-22-3329-2022, 2022
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We evaluate through first-order kinetic energy models, the minimum volume and mass of a pyroclastic density current generated at the Aso caldera that might affect any of five distal infrastructure sites. These target sites are all located 115–145 km from the caldera, but in well-separated directions. Our constraints of volume and mass are then compared with the scale of Aso-4, the largest caldera-forming eruption of Aso.
Albane Barbero, Roberto Grilli, Markus M. Frey, Camille Blouzon, Detlev Helmig, Nicolas Caillon, and Joël Savarino
Atmos. Chem. Phys., 22, 12025–12054, https://doi.org/10.5194/acp-22-12025-2022, https://doi.org/10.5194/acp-22-12025-2022, 2022
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The high reactivity of the summer Antarctic boundary layer results in part from the emissions of nitrogen oxides produced during photo-denitrification of the snowpack, but its underlying mechanisms are not yet fully understood. The results of this study suggest that more NO2 is produced from the snowpack early in the photolytic season, possibly due to stronger UV irradiance caused by a smaller solar zenith angle near the solstice.
Takahito Mitsui, Polychronis C. Tzedakis, and Eric W. Wolff
Clim. Past, 18, 1983–1996, https://doi.org/10.5194/cp-18-1983-2022, https://doi.org/10.5194/cp-18-1983-2022, 2022
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We provide simple quantitative models for the interglacial and glacial intensities over the last 800 000 years. Our results suggest that the memory of previous climate states and the time course of the insolation in both hemispheres are crucial for understanding interglacial and glacial intensities. In our model, the shift in interglacial intensities at the Mid-Brunhes Event (~430 ka) is ultimately attributed to the amplitude modulation of obliquity.
Helene M. Hoffmann, Mackenzie M. Grieman, Amy C. F. King, Jenna A. Epifanio, Kaden Martin, Diana Vladimirova, Helena V. Pryer, Emily Doyle, Axel Schmidt, Jack D. Humby, Isobel F. Rowell, Christoph Nehrbass-Ahles, Elizabeth R. Thomas, Robert Mulvaney, and Eric W. Wolff
Clim. Past, 18, 1831–1847, https://doi.org/10.5194/cp-18-1831-2022, https://doi.org/10.5194/cp-18-1831-2022, 2022
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The WACSWAIN project (WArm Climate Stability of the West Antarctic ice sheet in the last INterglacial) investigates the fate of the West Antarctic Ice Sheet during the last warm period on Earth (115 000–130 000 years before present). Within this framework an ice core was recently drilled at Skytrain Ice Rise. In this study we present a stratigraphic chronology of that ice core based on absolute age markers and annual layer counting for the last 2000 years.
Zhuang Jiang, Joel Savarino, Becky Alexander, Joseph Erbland, Jean-Luc Jaffrezo, and Lei Geng
The Cryosphere, 16, 2709–2724, https://doi.org/10.5194/tc-16-2709-2022, https://doi.org/10.5194/tc-16-2709-2022, 2022
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A record of year-round atmospheric nitrate isotopic composition along with snow nitrate isotopic data from Summit, Greenland, revealed apparent enrichments in nitrogen isotopes in snow nitrate compared to atmospheric nitrate, in addition to a relatively smaller degree of changes in oxygen isotopes. The results suggest that at this site post-depositional processing takes effect, which should be taken into account when interpreting ice-core nitrate isotope records.
Eric W. Wolff, Hubertus Fischer, Tas van Ommen, and David A. Hodell
Clim. Past, 18, 1563–1577, https://doi.org/10.5194/cp-18-1563-2022, https://doi.org/10.5194/cp-18-1563-2022, 2022
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Projects are underway to drill ice cores in Antarctica reaching 1.5 Myr back in time. Dating such cores will be challenging. One method is to match records from the new core against datasets from existing marine sediment cores. Here we explore the options for doing this and assess how well the ice and marine records match over the existing 800 000-year time period. We are able to recommend a strategy for using marine data to place an age scale on the new ice cores.
Julien Westhoff, Giulia Sinnl, Anders Svensson, Johannes Freitag, Helle Astrid Kjær, Paul Vallelonga, Bo Vinther, Sepp Kipfstuhl, Dorthe Dahl-Jensen, and Ilka Weikusat
Clim. Past, 18, 1011–1034, https://doi.org/10.5194/cp-18-1011-2022, https://doi.org/10.5194/cp-18-1011-2022, 2022
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We present a melt event record from an ice core from central Greenland, which covers the past 10 000 years. Our record displays warm summer events, which can be used to enhance our understanding of the past climate. We compare our data to anomalies in tree ring width, which also represents summer temperatures, and find a good correlation. Furthermore, we investigate an outstandingly warm event in the year 986 AD or 991 AD, which has not been analyzed before.
Saehee Lim, Meehye Lee, Joel Savarino, and Paolo Laj
Atmos. Chem. Phys., 22, 5099–5115, https://doi.org/10.5194/acp-22-5099-2022, https://doi.org/10.5194/acp-22-5099-2022, 2022
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We determined δ15N(NO3−) and Δ17O(NO3−) of PM2.5 in Seoul during 2018–2019 and estimated quantitatively the contribution of oxidation pathways to NO3− formation and NOx emission sources. The nighttime pathway played a significant role in NO3− formation during the winter, and its contribution further increased up to 70 % on haze days when PM2.5 was greater than 75 µg m−3. Vehicle emissions were confirmed as a main NO3− source with an increasing contribution from coal combustion in winter.
Zhuang Jiang, Becky Alexander, Joel Savarino, Joseph Erbland, and Lei Geng
The Cryosphere, 15, 4207–4220, https://doi.org/10.5194/tc-15-4207-2021, https://doi.org/10.5194/tc-15-4207-2021, 2021
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We used a snow photochemistry model (TRANSITS) to simulate the seasonal nitrate snow profile at Summit, Greenland. Comparisons between model outputs and observations suggest that at Summit post-depositional processing is active and probably dominates the snowpack δ15N seasonality. We also used the model to assess the degree of snow nitrate loss and the consequences in its isotopes at present and in the past, which helps for quantitative interpretations of ice-core nitrate records.
Helle Astrid Kjær, Lisa Lolk Hauge, Marius Simonsen, Zurine Yoldi, Iben Koldtoft, Maria Hörhold, Johannes Freitag, Sepp Kipfstuhl, Anders Svensson, and Paul Vallelonga
The Cryosphere, 15, 3719–3730, https://doi.org/10.5194/tc-15-3719-2021, https://doi.org/10.5194/tc-15-3719-2021, 2021
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Ice core analyses are often done in home laboratories after costly transport of samples from the field. This limits the amount of sample that can be analysed.
Here, we present the first truly field-portable continuous flow analysis (CFA) system for the analysis of impurities in snow, firn and ice cores while still in the field: the lightweight in situ analysis (LISA) box.
LISA is demonstrated in Greenland to reconstruct accumulation, conductivity and peroxide in snow cores.
Sarah Albertin, Joël Savarino, Slimane Bekki, Albane Barbero, and Nicolas Caillon
Atmos. Chem. Phys., 21, 10477–10497, https://doi.org/10.5194/acp-21-10477-2021, https://doi.org/10.5194/acp-21-10477-2021, 2021
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We report an efficient method to collect atmospheric NO2 adapted for multi-isotopic analysis and present the first NO2 triple oxygen and double nitrogen isotope measurements. Atmospheric samplings carried out in Grenoble, France, highlight the NO2 isotopic signature sensitivity to the local NOx emissions and chemical regimes. These preliminary results are very promising for using the combination of Δ17O and δ15N of NO2 as a probe of the atmospheric NOx emissions and chemistry.
Bette L. Otto-Bliesner, Esther C. Brady, Anni Zhao, Chris M. Brierley, Yarrow Axford, Emilie Capron, Aline Govin, Jeremy S. Hoffman, Elizabeth Isaacs, Masa Kageyama, Paolo Scussolini, Polychronis C. Tzedakis, Charles J. R. Williams, Eric Wolff, Ayako Abe-Ouchi, Pascale Braconnot, Silvana Ramos Buarque, Jian Cao, Anne de Vernal, Maria Vittoria Guarino, Chuncheng Guo, Allegra N. LeGrande, Gerrit Lohmann, Katrin J. Meissner, Laurie Menviel, Polina A. Morozova, Kerim H. Nisancioglu, Ryouta O'ishi, David Salas y Mélia, Xiaoxu Shi, Marie Sicard, Louise Sime, Christian Stepanek, Robert Tomas, Evgeny Volodin, Nicholas K. H. Yeung, Qiong Zhang, Zhongshi Zhang, and Weipeng Zheng
Clim. Past, 17, 63–94, https://doi.org/10.5194/cp-17-63-2021, https://doi.org/10.5194/cp-17-63-2021, 2021
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The CMIP6–PMIP4 Tier 1 lig127k experiment was designed to address the climate responses to strong orbital forcing. We present a multi-model ensemble of 17 climate models, most of which have also completed the CMIP6 DECK experiments and are thus important for assessing future projections. The lig127ksimulations show strong summer warming over the NH continents. More than half of the models simulate a retreat of the Arctic minimum summer ice edge similar to the average for 2000–2018.
Helle Astrid Kjær, Patrick Zens, Ross Edwards, Martin Olesen, Ruth Mottram, Gabriel Lewis, Christian Terkelsen Holme, Samuel Black, Kasper Holst Lund, Mikkel Schmidt, Dorthe Dahl-Jensen, Bo Vinther, Anders Svensson, Nanna Karlsson, Jason E. Box, Sepp Kipfstuhl, and Paul Vallelonga
The Cryosphere Discuss., https://doi.org/10.5194/tc-2020-337, https://doi.org/10.5194/tc-2020-337, 2021
Manuscript not accepted for further review
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We have reconstructed accumulation in 6 firn cores and 8 snow cores in Northern Greenland and compared with a regional Climate model over Greenland. We find the model underestimate precipitation especially in north-eastern part of the ice cap- an important finding if aiming to reconstruct surface mass balance.
Temperatures at 10 meters depth at 6 sites in Greenland were also determined and show a significant warming since the 1990's of 0.9 to 2.5 °C.
Seyedhamidreza Mojtabavi, Frank Wilhelms, Eliza Cook, Siwan M. Davies, Giulia Sinnl, Mathias Skov Jensen, Dorthe Dahl-Jensen, Anders Svensson, Bo M. Vinther, Sepp Kipfstuhl, Gwydion Jones, Nanna B. Karlsson, Sergio Henrique Faria, Vasileios Gkinis, Helle Astrid Kjær, Tobias Erhardt, Sarah M. P. Berben, Kerim H. Nisancioglu, Iben Koldtoft, and Sune Olander Rasmussen
Clim. Past, 16, 2359–2380, https://doi.org/10.5194/cp-16-2359-2020, https://doi.org/10.5194/cp-16-2359-2020, 2020
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We present a first chronology for the East Greenland Ice-core Project (EGRIP) over the Holocene and last glacial termination. After field measurements and processing of the ice-core data, the GICC05 timescale is transferred from the NGRIP core to the EGRIP core by means of matching volcanic events and common patterns (381 match points) in the ECM and DEP records. The new timescale is named GICC05-EGRIP-1 and extends back to around 15 kyr b2k.
Alexander H. Weinhart, Johannes Freitag, Maria Hörhold, Sepp Kipfstuhl, and Olaf Eisen
The Cryosphere, 14, 3663–3685, https://doi.org/10.5194/tc-14-3663-2020, https://doi.org/10.5194/tc-14-3663-2020, 2020
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From 1 m snow profiles along a traverse on the East Antarctic Plateau, we calculated a representative surface snow density of 355 kg m−3 for this region with an error less than 1.5 %.
This density is 10 % higher and density fluctuations seem to happen on smaller scales than climate model outputs suggest. Our study can help improve the parameterization of surface snow density in climate models to reduce the error in future sea level predictions.
Jean-Louis Bonne, Hanno Meyer, Melanie Behrens, Julia Boike, Sepp Kipfstuhl, Benjamin Rabe, Toni Schmidt, Lutz Schönicke, Hans Christian Steen-Larsen, and Martin Werner
Atmos. Chem. Phys., 20, 10493–10511, https://doi.org/10.5194/acp-20-10493-2020, https://doi.org/10.5194/acp-20-10493-2020, 2020
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This study introduces 2 years of continuous near-surface in situ observations of the stable isotopic composition of water vapour in parallel with precipitation in north-eastern Siberia. We evaluate the atmospheric transport of moisture towards the region of our observations with simulations constrained by meteorological reanalyses and use this information to interpret the temporal variations of the vapour isotopic composition from seasonal to synoptic timescales.
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Short summary
The ~ 74 ka eruption of Toba was one of the largest eruptions of the last 100 ka. We have measured the sulfur isotopic composition for 11 Toba eruption candidates in two Antarctic ice cores. Sulfur isotopes allow us to distinguish between large eruptions that have erupted material into the stratosphere and smaller ones that reach lower altitudes. Using this we have identified the events most likely to be Toba and place the eruption on the transition into a cold period in the Northern Hemisphere.
The ~ 74 ka eruption of Toba was one of the largest eruptions of the last 100 ka. We have...