Research article
03 Jul 2013
Research article | 03 Jul 2013
Towards a quasi-complete reconstruction of past atmospheric aerosol load and composition (organic and inorganic) over Europe since 1920 inferred from Alpine ice cores
S. Preunkert and M. Legrand
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Large mixing ratios of atmospheric nitrous acid (HONO) at Concordia (East Antarctic Plateau) in summer: a strong source from surface snow?
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Clim. Past, 10, 987–1000, https://doi.org/10.5194/cp-10-987-2014,https://doi.org/10.5194/cp-10-987-2014, 2014
Water-soluble organic carbon in snow and ice deposited at Alpine, Greenland, and Antarctic sites: a critical review of available data and their atmospheric relevance
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Fagerli, H., Legrand, M., Preunkert, S., Vestreng, V., Simpson, D., and Cerqueira, M.: Modeling historical long-term trends of sulfate, ammonium, and elemental carbon over Europe: A comparison with ice core records in the Alps, J. Geophys. Res., 112, D23S13, https://doi.org/10.1029/2006JD008044, 2007.
Guilhermet, J., Preunkert, S., Voisin, D., Baduel, C., and Legrand, M.: Major 20th century changes of water-soluble HUmic LIke Substances (HULIS$_WS$) aerosol over Europe inferred from Alpine ice cores, J. Geophys. Res., 118, 3869–3878, https://doi.org/10.1002/jgrd.50201, 2013.
Hammer, S., Wagenbach, D., Preunkert, S., Pio, C., Schlosser, C., and Meinhardt, F.: Lead-210 observations within CARBOSOL: A diagnostic tool for assessing the spatiotemporal variability of related chemical aerosol species?, J. Geophys. Res., 112, D23S03, https://doi.org/10.1029/2006JD008065, 2007.
Hering, S. and Cass, G.: The magnitude of bias in the measurement of PM2.5 arising from volatilisation of particulate nitrate from Teflon filters, J. Air Waste Manage., 49, 725–733, 1999.
Jenk, T. M., Szidat, S., Schwikowski, M., Gäggeler, H. W., Brütsch, S., Wacker, L., Synal, H.-A., and Saurer, M.: Radiocarbon analysis in an Alpine ice core: record of anthropogenic and biogenic contributions to carbonaceous aerosols in the past (1650–1940), Atmos. Chem. Phys., 6, 5381–5390, https://doi.org/10.5194/acp-6-5381-2006, 2006.
Kasper, A. and Puxbaum, H.: Seasonal variation of SO
2, HNO
3, NH
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Kiss, G., Varga, B., Galambos, I., and Ganszky, I.: Characterization of water-soluble organic matter isolated from atmospheric fine aerosol, J. Geophys. Res., 107, 8339, https://doi.org/10.1029/2001JD000603, 2002.
Lavanchy, V. M. H., Gäggeler, H. W., Schotterer, U., Schwikowski, M., and Baltensperger U.: Historical record of carbonaceous particle concentrations from a European high-alpine glacier (Colle Gnifetti, Switzerland), J. Geophys. Res., 104, 21227–21236, 1999.
Legrand, M., Preunkert, S., Wagenbach, D., and Fischer, H.: Seasonally resolved Alpine and Greenland ice core records of anthropogenic HCl Emissions over the 20th century, J. Geophys. Res., 107, 4139, https://doi.org/10.1029/2001JD001165, 2002.
Legrand, M., Preunkert, S., Wagenbach, D., Cachier, H., and Puxbaum, H.: A historical record of formate and acetate from a high elevation Alpine glacier: Implications for their natural versus anthropogenic budgets at the European scale, J. Geophys. Res., 108, 4788, https://doi.org/10.1029/2003JD003594, 2003.
Legrand, M., Preunkert, S., Galy-Lacaux, C., Liousse, C., and Wagenbach, D.: Atmospheric year-round records of dicarboxylic acids and sulfate at three French sites located between 630 and 4360 m elevation, J. Geophys. Res., 110, D13302, https://doi.org/10.1029/2004JD005515, 2005.
Legrand, M., Preunkert, S., Schock, M., Cerqueira, M., Kasper-Giebl, A., Afonso, J., Pio, C., Gelencsér, A., and Dombrowski-Etchevers, I.: Major 20th century changes of carbonaceous aerosol components (EC, WinOC, DOC, HULIS, carboxylic acids, and cellulose) derived from Alpine ice cores, J. Geophys. Res., 112, D23S11, https://doi.org/10.1029/2006JD008080, 2007a.
Legrand, M., Preunkert, S., Oliveira, T., Pio, C. A., Hammer, S., Gelencsér, A., Kasper-Giebl, A., and Laj, P.: Origin of C
2–C
5 dicarboxylic acids in the European atmosphere inferred from year-round aerosol study conducted at a west-east transect, J. Geophys. Res., 112, D23S07, https://doi.org/10.1029/2006JD008019, 2007b.
Legrand, M., Preunkert, S., May, B., Guilhermet, J., Hoffmann, H., and Wagenbach, D.: Major 20th century changes of the content and chemical speciation of organic carbon archived in Alpine ice cores: implications for the long-term change of organic aerosol over Europe, J. Geophys. Res., 118, 3879–3890, https://doi.org/10.1002/jgrd.50202, 2013.
May, B., Wagenbach, D., Hoffmann, H., Legrand, M., Preunkert, S., and Steier, P.: Constraints on the major sources of dissolved organic carbon in Alpine ice cores from Radiocarbon analysis over the bomb peak period, J. Geophys. Res., 118, 3319–3327, https://doi.org/10.1002/jgrd.50200, 2013.
Mylona, S.: Sulfur dioxide emissions in Europe 1880–1991, and their effect on sulphur concentrations and deposition, Tellus B, 48, 662–689, 1996.
Pio, C. A., Legrand, M., Oliveira, T., Afonso, J., Santos, C., Caseiro, A., Fialho, P., Barata, F., Puxbaum, H., Sanchez-Ochao, A., Kasper-Giebl, A., Gelencsér, A., Preunkert, S., Schock, M.: Climatology of aerosol composition (organic versus inorganic) at non-urban sites on a west-east transect across Europe, J. Geophys. Res., 112, D23S02, https://doi.org/10.1029/2006JD008038, 2007.
Preunkert, S.: L'histoire de la pollution atmosphérique Européenne reconstituée à partir des carottes de glace Alpine, Ph. D. thesis, 240 pp., Univ. Joseph Fourier de Grenoble, France, 2001.
Preunkert, S. and Wagenbach, D.: An automatic recorder for air/firn transfer studies of chemical aerosol species at remote glacier sites, Atmos. Environ., 32, 4021–4030, 1998.
Preunkert, S., Wagenbach, D., Legrand, M., and Vincent, C.: Col du Dôme (Mt Blanc Massif, French Alps) suitability for ice core studies in relation with past atmospheric chemistry over Europe, Tellus, 59, 993–1012, 2000.
Preunkert, S., Legrand, M., and Wagenbach, D.: Sulfate trends in a Col du Dôme (French Alps) ice core: A record of anthropogenic sulfate levels in the European mid-troposphere over the 20th century, J. Geophys. Res., 106, 31991–32004, 2001b.
Preunkert, S., Wagenbach, D., and Legrand, M.: A seasonally resolved Alpine ice core Record of Nitrate: Comparison with Anthropogenic Inventories and estimation of Pre-Industrial Emissions of NO from Europe, J. Geophys. Res., 108, 4681, https://doi.org/10.1029/2003JD003475, 2003.
Preunkert, S., Legrand, M., Jourdain, B., and Dombrowski-Etchevers, I.: Acidic gases (HCOOH, CH
3COOH, HNO
3, HCl, and SO
2) and related aerosol species at a high mountain Alpine site (4360 m elevation) in Europe, J. Geophys. Res., 112, D23S12, https://doi.org/10.1029/2006JD008225, 2007.
Preunkert, S., Legrand, M., Stricker, P., Bulat, S., Alekhina, I., Petit, J. R., Hoffmann, H., May, B., and Jourdain, B.: Quantification of Dissolved Organic Carbon at very low levels in natural ice samples by a UV induced oxidation method, Environ. Sci. Technol., 45, 673–678, 2011.
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Puxbaum, H. and Tscherwenka, W.: Relationship of major ions in snow fall and rime at Sonnblick observatoty (SBO, 3106 m) and implications for scavenging processes in mixed clouds, Atmos. Environ., 32, 4011–4020, 1998.
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Wagenbach, D., Preunkert, S., Schaefer, J., Jung, W., and Tomadin, L.: Northward transport of Saharan dust recorded in a deep Alpine ice core, in: The impact of African dust across the Mediterranean, edited by: Guerzoni, S. and Chester, R., Kluwer Academic Publishers, The Neetherlands, 291–300, 1996.
Wagenbach, D., Bohleber, P., and Preunkert, S.: Cold, Alpine ice bodies revisited: What may we learn from their impurity and isotope content?, Geogr. Ann. A, 94, 245–263, https://doi.org/10.1111/j.1468-0459.2012.00461.x, 2012.
